The Optics Laboratory
Group of
Hans Hallen, North Carolina State University Physics Department
The Probe
Fabrication -- Heat and Pull
Fabrication -- Etch
Fabrication -- Metal Coating
Throughput
Thermal Loading
New Ideas
Optical Properties, Theoretical
Early NSOM Efforts
L. Novotny, D.W. Pohl, P. Regli, Ultramicroscopy 57, 180-8 (1995).
Douglas A. Christensen, Ultramicroscopy 57, 189-95 (1995).
A perfectly conducting plane with a hole.
H.A. Bethe, Physical Review, 66, 163-182 (1944).
C.J. Bouwkamp, Phillips Res. Rep. 5, 401 (1950).
- Does a remarkable good job as observed in single molecule and our Raman studies.
A recent review
D. Barchiesi et al. Phys. Rev. E54 (4) pt B, 4285-92 (1996).
An interesting point:
L. Novotny, D.W. Pohl, B. Hecht, Ultramicr. 61 (1-4) 1-9 (1995).
L. Novotny, D.W. Pohl, B. Hecht, Opt. Lett. 20 (9) 970-2 (1995).
- Polarized light through an aperture has two spots of maximal electric field intensity.
- Polarized light through a (thinly) covered point has just one maxima, under the point.
Optical Properties, Experimental
Why do we coat the probe tip with metal?
To contain the light.
The modes do not remain localized to the dielectric core when it gets small.
M.A. Paesler and P.J. Moyer, "Near-Field Optics: Theory, Instrumentation and Applications," (Wiley, New York, 1996).
How well does the metal confine the light?
It depends upon the metal.
The light intensity falls exponentially into the metal, scaled by the penetration depth.
Aluminum is best at visible frequencies.
The minimum confined size for green light is ~10 nm.
E. Betzig, et al, Science, 251, 1468-1470 (1991).
How do we inspect the probes?
A point source Abbe pattern should be observed under a good optical microscope for both coated and uncoated fibers, otherwise throw the tip out.
Scanning electron microscopy - field emission e-gun for resolution - no conductive coating needed for tips - view aperture/shape at different angles
Fabrication of the Tapered Fiber Probe (Heat and Pull)
B.I. Yakobson, P.J. Moyer, M.A. Paesler, "Kinetic limits for sensing tip morphology in near-field scanning optical microscopes," J. Appl. Phys 73 (11) 7984-6 (1993).
G.A. Valaskovic, M. Holton, G.H. Morrison, "Parameter control, characterization, and optimization in the fabrication of optical fiber near-field probes," Appl. Opt. 34 (7) 1215 (1995).
R.L. Williamson, M.J. Miles, J. Appl. Phys. 80 (a) 4804-12 (1996).
Mufei Xiao et al, "Fabrication of Probe Tips for Reflection SNOM: Chemical Etch and Heating Pulling Methods," J. Vac. Sci. Tech. B15 (4) 1516 (1997).
Heat with a CO2 laser until the fiber begins to soften. Then pull hard (solenoid).
Heating power, timing, and pulling force are adjusted to give the desired tip shape.
The tip is coated with Aluminum while rotating. Inspection verifies lack of pinholes on shank
and presence of hole at tip (optical microscope).
Tip taper angle studied with optical or electron (SEM) microscopy.
In practice, a commercial tip puller is used.
An uncoated pulled (large to see details) tip:
Note the flat cleaved end which will define the aperture (up to diffusion of the evaporant metal).
Etching the fibers:
Basic (ammonium flouride) solutions give smooth surfaces.
Organic layers floating on the etchant use surface tension to provide controlled angle of the taper (30° for isooctane).
P. Hoffmann, B. Dutoit, and R.-P. Salathé, Ultramicroscopy 61, 165 (1995).
Etching based on properties of the core: S. Monobe and M Ohtsu, J. Lightwave Technol, 14 (10) 2231-5 (1996).
Advantages
High Throughput
Reproducible Shape
Disadvantages
Hard to get a well-defined aperture (no flat cleave as in heat&pull method)
Coating the fibers:
Standard technology.
Probe must be rotated -- usually a home-made holder.
Material
- Aluminum is best in the visible.
Thickness
- greater than a penetration depth.
- maximum set by film stability and by size of the probe.
- not critical.
- different than what the crystal monitor says due to rotation (~
p lower) and angle (cos q).
Coating the Probe with Aluminum
A coated probe (again large so the cleave/ aperture
are readily visible):
Coating Problem: Aluminum Diffusion
Polarization is effected by the lumps.
Solution -- Cool the Probe (Hallen Lab)
Radiation + Conduction
The Throughput Problem (Pulled fiber tips):
How important is spatial resolution to you?
It is very expensive in signal intensity.
Recall that one cannot arbitrarily increase the input power. Often one does not need the highest spatial resolution to take advantage of NSOM.
Other types of 'resolution'
Spectroscopic (cm-1)
Polarization (°)
These need high signal to noise so compete with spatial resolution.
Throughput Considerations:
Modeling for linear sections: ideaB.I. Yakobson and M.A. Paesler, "Tip optics for illumination NSOM: Extended zone approach," Ultramicroscopy 57, 204 (1995).
R = fiber radius,
f = taper angle, q = critical angle, r = tip aperture
The optical intensity decreases exponentially beyond (closer to tip than) cut-off, with length scale dependent upon geometry and material.
Damage of the probe:
Probe shape
(a)Before Damage
(b)After Damage
(c)A Model
(d)
Theory comes from ray tracing (count bounces/length):P.O. Boykin, M.A. Paesler, B.I. Yakobson, "Energy Dissipation in NSOM Probe
Fiber Tapers: Ray Tracing Assessment," SPIE Proceedings 2677, 148-153 (1996).
Tip Heating:
Due to imperfect reflections from the metal coating.
Be careful if you are not using Aluminum.
Results in metal diffusion to lumps and scattering loss of light (destroyed probe).
Measures of thermal time constant, models of probe temperature and profile, and thermal expansion of probe: A. LaRosa, B. I. Yakobson, and H.D. Hallen, APL 67, (18), 2597-2599 (1995).
Temperature profile from external Al reflectance D.I. Karaldjiev, R. Toledo-Crow and M. Vaez-Iravani, APL 67 (19) 2771-3 (1995).
Temperature profile from 'STM Thermocouple' M. Stahelin et al, APL 68 (19) 2603-5 (1996).
The experimental method
: A. LaRosa, B. I. Yakobson, and H.D. Hallen, "Origins and effects of thermal processes in near-field optical probes," APL 67, (18), 2597-2599 (1995).
Detect with a CW IR laser.
Measurements of the probe time constants:
slender probe with a 180 nm thick Al coating
2 mW red light, 1 mW of CW IR input triangles (after) and circles (before damage)
0.23 and 0.026 nW pk-pk Df
10.3 and 10.1 msec time constants Independent of details of probe shape.
Model suggests that several hundred microns
of the tip are heated above ambient
Peak is tens of microns from the tip.
New Ideas, two ways to increase the throughput by ~1000X:
Let Total Internal Reflection Work When it Can M.A. Paesler, H.D. Hallen, B.I. Yakobson, C.J. Jahncke, P.O. Boykin, and A. Meixner, "Near-field optical spectroscopy: enhancing the light budget," Microscopy and Microanalysis 3, 815 (1997).
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Last updated on September 27, 2000